Towards weighing individual atoms by high-angle scattering of electrons

Author(s)
Giacomo Argentero, Clemens Mangler, Jani Kotakoski, Franz Eder, Jannik C. Meyer
Abstract

We consider theoretically the energy loss of electrons scattered to high angles when assuming that the primary beam can be limited to a single atom. We discuss the possibility of identifying the isotopes of light elements and of extracting information about phonons in this signal. The energy loss is related to the mass of the much heavier nucleus, and is spread out due to atomic vibrations. Importantly, while the width of the broadening is much larger than the energy separation of isotopes, only the shift in the peak positions must be detected if the beam is limited to a single atom. We conclude that the experimental case will be challenging but is not excluded by the physical principles as far as considered here. Moreover, the initial experiments demonstrate that the separation of gold and carbon based on a signal that is related to their mass, rather than their atomic number.

Organisation(s)
Physics of Nanostructured Materials
Journal
Ultramicroscopy
Volume
151
Pages
23–30
No. of pages
8
ISSN
0304-3991
Publication date
12-2014
Peer reviewed
Yes
Austrian Fields of Science 2012
210006 Nanotechnology, 103008 Experimental physics, 103009 Solid state physics
Keywords
ASJC Scopus subject areas
Electronic, Optical and Magnetic Materials, Instrumentation, Atomic and Molecular Physics, and Optics
Portal url
https://ucrisportal.univie.ac.at/en/publications/towards-weighing-individual-atoms-by-highangle-scattering-of-electrons(814ac4ed-7cc6-4926-8634-0e2b796a30d6).html