Atomic structure from large-area, low-dose exposures of materials

Author(s)
Jannik C. Meyer, Jani Kotakoski, Clemens Mangler
Abstract

Beam-induced structural modifications are a major nuisance in the study of materials by high-resolution electron microscopy. Here, we introduce a new approach to circumvent the radiation damage problem by a statistical treatment of large, noisy, low-dose data sets of non-periodic configurations (e.g. defects) in the material. We distribute the dose over a mixture of different defect structures at random positions and with random orientations, and recover representative model images via a maximum likelihood search. We demonstrate reconstructions from simulated images at such low doses that the location of individual entities is not possible. The approach may open a route to study currently inaccessible beam-sensitive configurations.

Organisation(s)
Physics of Nanostructured Materials
Journal
Ultramicroscopy
Volume
145
Pages
13-21
No. of pages
9
ISSN
0304-3991
DOI
https://doi.org/10.1016/j.ultramic.2013.11.010
Publication date
12-2013
Peer reviewed
Yes
Austrian Fields of Science 2012
210006 Nanotechnology, 103008 Experimental physics, 103009 Solid state physics
Keywords
ASJC Scopus subject areas
Electronic, Optical and Magnetic Materials, Instrumentation, Atomic and Molecular Physics, and Optics
Portal url
https://ucrisportal.univie.ac.at/en/publications/atomic-structure-from-largearea-lowdose-exposures-of-materials(55cfd028-5caf-469f-b1f5-1b395b000799).html